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Estimating regional carbon (C) stocks and understanding their dynamics is crucial, both from the perspective of sustainable landscape management and global change feedback. This study combines remote sensing techniques and a coupled GIS-CENTURY model to estimate regional biomass C stocks and SOC dynamics for Guiera senegalensis shrub communities in Senegal's Peanut Basin. A statistical model relating field-measured shrub aboveground biomass C at training plots to satellite image-derived shrub abundances was developed and used to estimate regional biomass C across a major part of the Basin. Regional SOC dynamics were modeled by coupling the CENTURY model and GIS databases. Significant correlation (r =0.73; p =0.05) was observed between aboveground biomass C and satellite image-derived shrub abundance at the training plots. Aboveground biomass C stocks ranged from 0.01 to 0.45Mgha⁻¹ with an approximate total of 247,000MgC for the 3060km² study area. CENTURY model predictions indicate that C sequestration in these systems is contingent on long-term effectiveness of non-thermal management of shrub residue and that the actual rates depend strongly on soil type and scenarios of future land management. Compared with the traditional “pruning-burned” management practice, returning prunings for 50 years would increase soil C sequestration by 200-350% without fertilization, and increase soil C sequestration by 270-483% under a low (35kgha⁻¹ Nyr⁻¹; 20kgha⁻¹ Pyr⁻¹) fertilization regime, depending on soil type and climate conditions. These results indicate that altered land management could contribute to transforming these degraded semiarid agroecosystems from a source to a sink for atmospheric CO₂.